Accelerator mass spectrometry (AMS) for beryllium-7 measurements in smallest rainwater samples

authored by
Collin Tiessen, Daniel Bemmerer, Georg Rugel, Rebecca Querfeld, Andreas Scharf, Georg Steinhauser, Silke Merchel
Abstract

Beryllium-7, mainly measured via γ-spectrometry, is used as a (natural) radiotracer for education and science. For activities < 0.1 Bq and samples containing also longer-lived 10 Be, accelerator mass spectrometry (AMS) is the method-of-choice. We demonstrate that 7 Be and 10 Be can be quantified at the Dresden AMS facility on the same prepared BeO. Detection limits ( 7 Be) are ~ 0.6 mBq. Samples as small as tens of millilitres of rainwater can be chemically processed (after acidification) within a few hours without expensive and slow ion exchange. Isobar ( 7 Li) suppression by chemistry and AMS is sufficient to guarantee for an ultrasensitive, cheap, and fast detection method for 7 Be allowing high sample throughput.

Organisation(s)
Centre for Radiation Protection and Radioecology
External Organisation(s)
Helmholtz-Zentrum Dresden-Rossendorf (HZDR)
University of Ottawa
Type
Article
Journal
Journal of Radioanalytical and Nuclear Chemistry
Volume
319
Pages
965-973
No. of pages
9
ISSN
0236-5731
Publication date
15.03.2019
Publication status
Published
Peer reviewed
Yes
ASJC Scopus subject areas
Analytical Chemistry, Nuclear Energy and Engineering, Radiology Nuclear Medicine and imaging, Pollution, Spectroscopy, Public Health, Environmental and Occupational Health, Health, Toxicology and Mutagenesis
Sustainable Development Goals
SDG 3 - Good Health and Well-being
Electronic version(s)
https://doi.org/10.1007/s10967-018-6371-6 (Access: Closed)